研究中心

地-气界面科学中心

1. 科研项目

新增项目:

1)国家自然科学基金委员会创新研究群体,地-气界面过程及环境气候效应,2023.01-2027.12. 负责人:傅平青

2)国家自然科学基金,面上项目,大气氨-铵气/粒转化过程及氮来源的氮同位素示踪研究,2023.01-2026.12. 负责人:李晓东

3)国家自然科学基金,面上项目,高浓度NOx环境下棕碳水溶性含N和含S有机物的非均相二次形成与转化及其光学特性的变化规律,2023.01-2026.12. 负责人:Chandra Mouli Pavuluri

4)国家重点研发计划青年科学家项目,海-气系统与海洋有机气溶胶相互作用过程与机理研究,2023.01-2027.12,负责人:朱佳雷

5)国家自然科学基金,面上项目,森林大气棕碳气溶胶光学特性及其影响机制的分子水平研究,2023.01-2026.12. 负责人:邓君俊

6)国家自然科学基金,青年项目,华北晚古生代煤中丝质体碳同位素原位分析及分馏机理研究,2023.01-2025.12. 负责人:徐占杰

7)国家自然科学基金,青年项目,天津市大气边界层中有机硫气溶胶的垂直分布特征研究,2023.01-2025.12. 负责人:谢巧蓉

已有项目:

8) 国家杰出青年科学基金项目,气溶胶化学,2017.01-2021.12. 负责人:傅平青

9) 国家自然科学基金,重大研究计划合作子项目,二次有机气溶胶液相生成机制和化学过程的碳氮稳定同位素研究,2017.01-2019.12. 负责人:Chandra Mouli Pavuluri

10) 国家自然科学基金,面上项目,利用氮氧同位素组成辨识汽车尾气来源的城市气溶胶硝酸盐,2018.01-2021.12. 负责人:李晓东

11) 国家自然科学基金,面上项目,天津市有机气溶胶的人为和生物源贡献、大气过程及季节性变化研究,2018.01-2021.12. 负责人:Chandra Mouli Pavuluri

12) 国家自然科学基金,面上项目,东印度洋海域大气气溶胶中生物标志物的特征、来源与影响因素,2020.01-2023.12,负责人:胡伟

13) 国家自然科学基金,应急管理项目,天津市气溶胶中二元酸及其稳定碳同位素组成研究,2017.01-2018.12. 负责人:Chandra Mouli Pavuluri

14) 国家重点研发计划重点专项子课题,大气二次颗粒形成和老化过程中有机单体同位素分馏机制,2017.12-2020.11. 负责人:Chandra Mouli Pavuluri

15) 国家重点研发计划项目,子课题,全球高时空分辨率气溶胶数据集,2019.01-2021.12. 负责人:邓君俊

16) 国家自然科学基金,青年科学基金项目,印度洋海域大气气溶胶和海洋微表层中细菌的特征及其冰核活性,2019.01-2021.12,负责人:胡伟

17) 国家自然科学基金,青年项目,城市和高山大气气溶胶中游离态和结合态氨基酸的单体氮同位素研究,2020.01-2022.12. 负责人:吴礼彬

18) 国家自然科学基金,青年项目,天津市大气细颗粒物中脂类化合物的单体稳定碳同位素研究,2019.01-2021.12. 负责人:任露洁

19) 国家自然科学基金,国际(地区)合作与交流项目,华北沿海地区大气有机-无机气溶胶耦合演变:对二次有机气溶胶形成的影响,2019.03-2022.02,负责人:傅平青

2. 发表文章(2019年至今)

1) Qiang Zhang, Wei Hu, Hong Ren, Jianbo Yang, Junjun Deng, Dawei Wang, Yele Sun, Zifa Wang, Kimitaka Kawamura, Pingqing Fu. Diurnal variations in primary and secondary organic aerosols in an eastern China coastal city: The impact of land-sea breezes. Environmental Pollution 2023,319.121016.

2) Shujun Zhong, Shuang Chen, Junjun Deng, Yanbing Fan, Qiang Zhang, Qiaorong Xie, Yulin Qi, Wei Hu, Libin Wu, Xiaodong Li, Chandra Mouli Pavuluri, Jialei Zhu, Xin Wang, Di Liu, Xiaole Pan, Yele Sun, Zifa Wang, Yisheng Xu, Haijie Tong, Hang Su, Yafang Cheng, Kimitaka Kawamura, Pingqing Fu. Impact of biogenic secondary organic aerosol (SOA) loading on the molecular composition of wintertime PM2.5 in urban Tianjin: an insight from Fourier transform ion cyclotron resonance mass spectrometry. Atmospheric Chemistry and Physics 2023,23(3),2061-2077.

3) Libin Wu, Ming Sheng, Xiaodong Liu, Zhangqin Zheng, Steven D Emslie, Ning Yang, Xueying Wang, Yaguang Nie, Jing Jin, Qiaorong Xie, Shuang Chen, Donghuan Zhang, Sihui Su, Shujun Zhong, Wei Hu, Junjun Deng, Jialei Zhu, Yulin Qi, Cong-Qiang Liu, Pingqing Fu. Molecular transformation of organic nitrogen in Antarctic penguin guano-affected soil. Environment International 2023,172, 107796.

4) Peimin Duan, Wei Hu, Zhijun Wu, Kai Bi, Jialei Zhu, Pingqing Fu. Ice nucleation activity of airborne pollen: A short review of results from laboratory experiments. Atmospheric Research 2023,106659.

5) Subba Rao Devineni, Chandra Mouli Pavuluri, Shuang Wang, Lujie Ren, Zhanjie Xu, Peisen Li, Pingqing Fu undefinedamp; Cong-Qiang Liu. Size-resolved characteristics and sources pf inorganic ions, carbonaceous components and dicarboxylic acids, benzoic acids, oxocarboxylic acids and α-dicarbonyls in wintertime aerosols from Tianjin, North China. Aerosol Science and Engineering, 2023. https://doi.org/10.1007/s41810-022-00159-0

6) Zhichao Dong, Chandra Mouli Pavuluri, Zhanjie Xu, Yu Wang, Peisen Li, Pingqing Fu, undefinedamp; Cong-Qiang Liu. Measurement report: Chemical components and 13C and 15N isotope ratios of fine aerosols over Tianjin, North China: year-round observations. Atmospheric Chemistry and Physics 2023,23, 2119-2143. https://doi.org/10.5194/acp-23-2119-2023

7)Shiyuan Ding, Yingying Chen, Qinkai Li, Xiao-Dong Li. Using stable sulfur isotope to trace sulfur oxidation pathways during the winter of 2017-2019 in Tianjin, North China. International Journal of Environmental Research and Public Health 2022,10966.

8)Yulin Qi, Qiaorong Xie, Jun-Jian Wang, Ding He, Hongyan Bao, Qing-Long Fu, Sihui Su, Ming Sheng, Si-Liang Li, Dietrich A Volmer, Fengchang Wu, Guibin Jiang, Cong-Qiang Liu, Pingqing Fu. Deciphering dissolved organic matter by Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS): from bulk to fractions and individuals. Carbon Research 2022, 1(1), 1-22.

9)Xueyan Zhao, Zhanjie Xu, Peisen Li, Zhichao Dong, Pingqing Fu, Cong-Qiang Liu, Chandra Mouli Pavuluri. Characteristics and seasonality of trace elements in fine aerosols from Tianjin, North China during 2018-2019. Environmental Advances 2022, 9: 100263.

10)Peisen Li, Chandra Mouli Pavuluri, Zhichao Dong, Zhanjie Xu, Pingqing Fu, Cong-Qiang Liu. Year-round observations of stable carbon isotopic composition of carboxylic acids, oxoacids and α-Dicarbonyls in fine aerosols at Tianjin, North China: Implications for origins and aging. Science of The Total Environment 2022, 834: 155385.

11)Sihui Su, Qiaorong Xie, Alan J Smith, Yunchao Lang, Wei Hu, Dong Cao, Siyao Yue, Shuang Chen, Jialei Zhu, Yisheng Xu, Nicholle GA Bell, Dušan Uhrín, Pingqing Fu. A New Structural Classification Scheme for Dissolved Organic Sulfur in Urban Snow from North China. Environmental Science undefinedamp; Technology Letters 2022, 9(5), 366-374.

12)Qiaorong Xie, Sihui Su, Yuqing Dai, Wei Hu, Siyao Yue, Dong Cao, Guibin Jiang, Pingqing Fu. Deciphering 13C and 34S Isotopes of Organosulfates in Urban Aerosols by FT-ICR Mass Spectrometry. Environmental Science undefinedamp; Technology Letters 2022, 9(6), 526-532.

13)Siyao Yue, Linjie Li, Weiqi Xu, Jian Zhao, Hong Ren, Dongsheng Ji, Ping Li, Qiang Zhang, Lianfang Wei, Qiaorong Xie, Xiaole Pan, Zifa Wang, Yele Sun, Pingqing Fu. Biological and Nonbiological Sources of Fluorescent Aerosol Particles in the Urban Atmosphere. Environmental Science undefinedamp; Technology 2022, https://doi.org/10.1021/acs.est.1c07966

14)Wan Wei, Qiaorong Xie, Qin Yan, Wei Hu, Shuang Chen, Sihui Su, Donghuan Zhang, Li Wu, Shu Huang, Shujun Zhong, Junjun Deng, Ting Yang, Jie Li, Xiaole Pan, Zifa Wang, Yele Sun, Shaofei Kong, Pingqing Fu. Dwindling aromatic compounds in fine aerosols from chunk coal to honeycomb briquette combustion. Science of The Total Environment 2022,838,155971.

15)Hong Ren, Wei Hu, Siyao Yue, Libin Wu, Lujie Ren, Xiaole Pan, Zifa Wang, Yele Sun, Kimitaka Kawamura, Pingqing Fu. Tracer-based characterization of fine carbonaceous aerosol in Beijing during a strict emission control period. Science of The Total Environment 2022, 841, 156638.

16)Jialei Zhu, Joyce E Penner*, Anne Garnier, Olivier Boucher, Meng Gao, Lei Song, Junjun Deng, Cong‐Qiang Liu, Pingqing Fu. Decreased aviation leads to increased ice crystal number and a positive radiative effect in cirrus clouds. AGU Advances 2022, 3(2), e2021AV000546.

17)Ding, Shiyuan, Chen, Yingying, Devineni, Subba Rao, Pavuluri, Chandra Mouli, Li, Xiao-Dong. Distribution characteristics of organosulfates (OSs) in PM2.5 in Tianjin, Northern China: Quantitative analysis of total and three OS species. Science of The Total Environment 2022, 834. 155314.

18)Xiao, H., Ding, S.-Y., Ji, C.-W., Li, Q.-K. and Li, X.-D. Combustion related ammonia promotes PM2.5 accumulation in autumn in Tianjin, China. Atmospheric Research 2022, 275, 106225.

19)Yang, M., Liu, C.-Q., Li, X.-D., Ding, S., Cui, G., Teng, H.H., Lv, H., Wang, Y., Zhang, X. and Guan, T. Carbonsulfur coupling in a seasonally hypoxic, high-sulfate reservoir in SW China: Evidence from stable CS isotopes and sulfate-reducing bacteria. The Science of the total environment 2022, 828, 154537-154537.

20)Donghuan Zhang, Hong Ren, Wei Hu, Libin Wu, Lujie Ren, Junjun Deng, Qiang Zhang, Yele Sun, Zifa Wang, Kimitaka Kawamura, Pingqing Fu. Latitudinal difference in the molecular distributions of lipid compounds in the forest atmosphere in China. Environmental Pollution 2022,294,118578.

21)Huixia Han, Yujie Feng, Jing Chen, Qiaorong Xie, Shuang Chen, Ming Sheng, Shujun Zhong, Wan Wei, Sihui Su, Pingqing Fu. Acidification impacts on the molecular composition of dissolved organic matter revealed by FT-ICR MS. Science of the Total Environment 2021, 805,150284. DOI:10.1016/j.scitotenv.2021.150284.

22)Junjun Deng, Hao Ma, Xinfeng Wang, Shujun Zhong, Zhimin Zhang, Jialei Zhu, Yanbing Fan, Wei Hu, Libin Wu, Xiaodong Li, Lujie Ren, Chandra Mouli Pavuluri, Xiaole Pan, Yele Sun, Zifa Wang, Kimitaka Kawamura, Pingqing Fu. Measurement Report: Optical properties and sources of water-soluble brown carbon in Tianjin, North China: insights from organic molecular compositions. Atmospheric Chemistry and Physics, 2022, 22(10): 6449-6470. https://doi.org/10.5194/acp-2021-1045.、23)Shuang Chen, Qiaorong Xie, Sihui Su, Libin Wu, Shujun Zhong, Zhimin Zhang, Chao Ma, Yulin Qi, Wei Hu, Junjun Deng, Lujie Ren, Dongqiang Zhu, Qingjun Guo, Cong-Qiang Liu, Kyoung-Soon Jang, Pingqing Fu. Source and formation process impact the chemodiversity of rainwater dissolved organic matter along the Yangtze River Basin in summer. Water research 2022,211,118024.

24)Tenglong Shi, Jiecan Cui, Dongyou Wu, Yuxuan Xing, Yang Chen, Yue Zhou, Wei Pu, Xin Wang. Snow albedo reductions induced by the internal/external mixing of black carbon and mineral dust, and different snow grain shapes across northern China, Environmental Research 2022,208,112670, https://doi.org/10.1016/j.envres.2021.112670

25)Siyao Yue, Jialei Zhu, Shuang Chen, Qiaorong Xie, Wei Li, Linjie Li, Hong Ren, Sihui Su, Ping Li, Hao Ma, Yanbing Fan, Borong Cheng, Libin Wu, Junjun Deng, Wei Hu, Lujie Ren, Lianfang Wei, Wanyu Zhao, Yu Tian, Xiaole Pan, Yele Sun, Zifa Wang, Fengchang Wu, Cong-Qiang Liu, Hang Su, Joyce E. Penner, Ulrich Pöschl, Meinrat O. Andreae, Yafang Cheng, Pingqing Fu. Brown carbon from biomass burning imposes strong circum-Arctic warming. One Earth 2022,5(3),293-304.DOI: 10.1016/j.oneear.2022.02.006.

26)Mengdi Yang, Cong-Qiang Liu, Xiao-Dong Li, Shiyuan Ding, Gaoyang Cui, Hui Henry Teng, Hong Lv, Xuecheng Zhang, Tianhao Guan. Carbonsulfur coupling in a seasonally hypoxic, high-sulfate reservoir in SW China: Evidence from stable C-S isotopes and sulfate-reducing bacteria. Science of The Total Environment 2022,828,154537. https://doi.org/10.1016/j.scitotenv.2022.154537

27)Su, S., Xie, Q., Lang, Y., Cao, D., Xu, Y., Chen, J., Chen, S., Hu, W., Qi, Y., Pan, X., Sun, Y., Wang, Z., Liu, C., Jiang, G., Fu, P. High Molecular Diversity of Organic Nitrogen in Urban Snow in North China. Environmental Science undefinedamp; Technology 2021, https://doi.org/10.1021/acs.est.0c06851

28)Wu, L., Yue, S., Shi, Z., Hu, W., Chen, J., Ren, H., Deng, J., Ren, L., Fang, Y., Yan, H., Li, W., Harrison, R., Fu, P. Source forensics of inorganic and organic nitrogen using δ15N for tropospheric aerosols over Mt. Tai. npj Climate and Atmospheric Science 2021, DOI: 10.1038/s41612-021-00163-0

29)Huang, S., Hu, W., Chen, J., Wu, Z., Zhang, D., Fu, P. Overview of biological ice nucleating particles in the atmosphere. Environment International 2021, 146, 106197. https://doi.org/10.1016/j.envint.2020.106197

30)Pavuluri, C., Wang, S., Fu, P., Zhao, W., Xu, Z., Liu, C. Molecular Distributions of Diacids, Oxoacids, and α-Dicarbonyls in Summer-and Winter-Time Fine Aerosols from Tianjin, North China: Emissions from Combustion Sources and Aqueous Phase Secondary Formation. Journal of Geophysical Research: Atmospheres 2021, https://doi.org/10.1029/2020JD032961

31)Li, P., Pavuluri, C. M., Dong, Z., Xu, Z., Wang, Y., Fu, P., undefinedamp; Liu, C.-Q., Characteristics, seasonality, and secondary formation processes of diacids and related compounds in fine aerosols during warm and cold periods: Year-round observations at Tianjin, North China. Journal of Geophysical Research: Atmospheres 2021, e2021JD035435. https://doi.org/10.1029/2021JD035435

32)Hu, W., Liu, D., Su, S., Ren, L., Ren, H., Wei, L., Yue, S., Xie, Q., Zhang, Z., Wang, Z., Yang, N., Wu, L., Deng, J., Qi, Y., Fu, P., Photochemical Degradation of Organic Matter in the Atmosphere. Advanced Sustainable Systems 2021. DOI: 10.1002/adsu.202100027

33)Cui, G., Li, X., Li, S., Ding, S., Li, Q., Yang, M., Lv, H., Wang, Y. Varying water column stability controls the denitrification process in a subtropical reservoir, Southwest China. Journal of Environmental Sciences 2021, 111,208-219.

34)Cui, G., Wang, B., Xiao, J., Qiu, X., Liu, C., Li, X., Water column stability driving the succession of phytoplankton functional groups in karst hydroelectric reservoirs. J. Hydrol. 2021, 592, 125607.

35)Han, H., Feng, Y., Chen, J., Xie, Q., Chen, S., Sheng, M., Zhong, S., Wei, W., Su, S., Fu, P. Acidification impacts on the molecular composition of dissolved organic matter revealed by FT-ICR MS. Science of the Total Environment 2021, 805,150284. DOI:10.1016/j.scitotenv.2021.150284.

36)Zhang, Z., Zhao, W., Hu, W., Deng, J., Ren, L., Wu, L., Chen, S., Meng, J., Pavuluri, C., Sun, Y., Wang, Z., Kawamura, K., Fu, P. Molecular characterization and spatial distribution of dicarboxylic acids and related compounds in fresh snow in China. Environmental Pollution 2021, 291, 118114. DOI: 10.1016/j.envpol.2021.118114.

37)Ren, H., Hu, W., Wei, L., Yue, S., Zhao, J., Li, L., Wu, L., Zhao, W., Ren, L., Kang, M., Xie, Q., Su, S., Pan, X., Wang, Z., Sun, Y., Kawamura, K., Fu, P. Measurement report: Vertical distribution of biogenic and anthropogenic secondary organic aerosols in the urban boundary layer over Beijing during late summer. Atmospheric Chemistry and Physics 2021, 21, 12949-12963.  DOI: 10.5194/acp-21-12949-2021.

38)Xie, Q., Su, S., Chen, J., Dai, Y., Yue, S., Su, H., Tong, H., Zhao, W., Ren, L., Xu, Y., Cao, D., Li, Y., Sun, Y., Wang, Z., Liu, C., Kawamura, K., Jiang, G., Cheng, Y., Fu, P. Increase of nitrooxy organosulfates in firework-related urban aerosols during Chinese New Year's Eve. Atmospheric Chemistry and Physics 2021, 21, 14, 11453-11465. DOI: 10.5194/acp-21-11453-2021.

39)Zhang, X., Ding, S., Lv, H., Cui, G., Yang, M., Wang, Y., Guan, T., Li, X., Microbial controls on heavy metals and nutrients simultaneous release in a seasonally stratified reservoir. Environ Sci Pollut Res 2021, Res. 15776.

40)Ding, S., Wang, Y., Yang, M., Shi, R., Ma, T., Cui, G. and Li, X., Distribution and speciation of arsenic in seasonally stratified reservoirs: Implications for biotransformation mechanisms governing interannual variability. Science of the total environment 2021, 150925-150925.

41)Niu, M., Hu, W., Cheng, B., Wu, L., Ren, L., Deng, J., Shen, F., and Fu, P., Influence of rainfall on fungal aerobiota in the urban atmosphere over Tianjin, China: A case study. Atmospheric Environment:X 2021, X 12: 100137.

42)Wang, Z., Hu, W., Niu, H., Hu, W., Xu, Y., Wu, L., Ren, L., Deng, J., Guo, S., Wu, Z., Zhang, D., Fu, P., and Hu, M., Variations in physicochemical properties of airborne particles during a heavy haze-to-dust episode in Beijing. Science of The Total Environment. 2021, 762: 143081–143081.

43)Deng, J., Gao, Y., Zhu,J., Li, L., Yu, S., Kawamura, K., and Fu, P., Molecular markers for fungal spores and biogenic SOA over the Antarctic Peninsula: Field measurements and modeling results. Science of the Total Environment 2021, 762, 143089.

44) Xu, S.F., L.J. Ren, Y.C. Lang*, S.J. Hou, H. Ren, LF. Wei, L.B. Wu, J.J. Deng, W. Hu, X.L. Pan, Y.L. Sun, Z.F. Wang, H. Su, Y.F. Cheng, and P.Q. Fu. Molecular markers of biomass burning and primary biological aerosols in urban Beijing: Size distribution and seasonal variation. Atmospheric Chemistry and Physics 2020,20, 3623–3644.

45) Fan, Y.B., C.-Q. Liu, L.J. Li, L.J. Ren, H. Ren, W. Hu, J.J. Deng, L.B. Wu, S.J. Zhong, Y. Zhao, S. Wang, C.M. Pavuluri, X.L. Pan, Y.L. Sun, Z.F. Wang, and P.Q. Fu. Molecular characterization and seasonal variation in primary and secondary organic aerosols in Tianjin, China. Atmospheric Chemistry and Physics 2020,20(1), 117–137.

46) Wang, X., X. Zhang, and W. Di. Development of an improved two-sphere integration technique for quantifying black carbon concentrations in the atmosphere and seasonal snow. Atmos. Meas. Tech. 2020, 13, 39–52.

47) Deng, J., Zhao, W., Wu, L., Hu, W., Ren, L., Wang, X., and P.Q. Fu. Black carbon in Xiamen, China: Temporal variations, transport pathways and impacts of synoptic circulation. Chemosphere 2020, 241, 125133.

48) Ren, L.J., Y.Y. Wang, K. Kawamura, S. Bikkina, N. Haghipour, L. Wacker, C.M. Pavuluri, Z.M. Zhang, S.Y. Yue, Y.L. Sun, Z.F. Wang, X.J. Feng, C.-Q. Liu, T.I. Eglinton, and P.Q. Fu. Source forensics of n-alkanes and fatty acids in urban aerosols using compound specific radiocarbon/stable carbon isotopic composition. Environmental Research Letters 2020. DOI: 10.1088/1748-9326/ab8333.

49) Feng, X., Q. Li, Y. Tao, S. Ding, Y. Chen, and X.-D. Li. Impact of Coal Replacing Project on atmospheric fine aerosol nitrate loading and formation pathways in urban Tianjin: Insights from chemical composition and N-15 and O-18 isotope ratios. Science of the Total Environment 2020, 708, 134797.

50) Hu, W., Wang, Z., Huang, S., Ren, L., Yue, S., Li, P., Xie, Q., Zhao, W., Wei, L., Ren, H., Wu, L., Deng, J., and P.Q. Fu. Biological Aerosol Particles in Polluted Regions. Current Pollution Reports 2020. https://doi.org/10.1007/s40726-020-00138-4

51) Ren, L.J., W. Hu, J.Z. Hou, L.J. Li, S.Y. Yue, Y.L. Sun, Z.F. Wang, X.D. Li, C.M. Pavuluri, S.J. Hou, C.-Q. Liu, K. Kawamura, R.M. Ellam, and P.Q. Fu. Compound-specific stable carbon isotope ratios of terrestrial biomarkers in urban aerosols from Beijing, China. ACS Earth and Space Chemistry 2019,3(9), 1896–1904.

52) Ding, S., Zhang, L., Li, Y., Hou, L. Fabrication of a novel polyvinylidene fluoride membrane via binding SiO2 nanoparticles and a copper ferrocyanide layer onto a membrane surface for selective removal of cesium. J. Hazard. Mater. 2019,368,292-299.

53) Wu, L., Ren, H., Wang, P., Chen, J., Fang, Y., Hu, W., Ren, L., Deng, J., Song, Y., Li, J., Sun, Y., Wang, Z., Liu, C.Q., Ying, Q. and Fu, P.Q. (2019) Aerosol Ammonium in the Urban Boundary Layer in Beijing: Insights from Nitrogen Isotope Ratios and Simulations in Summer 2015. Environmental Science and Technology Letters 2019,6(7): 389–395.

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